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Modeling assessment of air emission flux of mercury from soils in terrestrial landscape components: Model tests and sensitivities

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dc.contributor.author Tsiros, IX en
dc.date.accessioned 2014-06-06T06:44:52Z
dc.date.available 2014-06-06T06:44:52Z
dc.date.issued 2002 en
dc.identifier.issn 1047-3289 en
dc.identifier.uri http://62.217.125.90/xmlui/handle/123456789/2112
dc.subject.classification Engineering, Environmental en
dc.subject.classification Environmental Sciences en
dc.subject.classification Meteorology & Atmospheric Sciences en
dc.subject.other MUNICIPAL SEWAGE-SLUDGE en
dc.subject.other ELEMENTAL MERCURY en
dc.subject.other GASEOUS MERCURY en
dc.subject.other ATMOSPHERE en
dc.subject.other DEPOSITION en
dc.subject.other WATER en
dc.subject.other CATCHMENTS en
dc.subject.other EXCHANGE en
dc.subject.other SURFACE en
dc.subject.other HG en
dc.title Modeling assessment of air emission flux of mercury from soils in terrestrial landscape components: Model tests and sensitivities en
heal.type journalArticle en
heal.language English en
heal.publicationDate 2002 en
heal.abstract The abilities of a screening-level model to predict variations in elemental mercury (Hg-0) air emissions from soils in terrestrial landscapes are examined by comparing simulation results to published observational data and by performing sensitivity analyses. Despite uncertainties and simplifications, the model results obtained offer some degree of confidence in the model's joint ability to relate readily available environmental parameters to airborne emissions of Hg predicted by coupling simple atmospheric and soil parameters with Hg cycling and transport algorithms. The model reasonably predicted the observational data in the considered data sets except for one site for which significant uncertainty was associated with model input data. Predictions are consistent with many trends observed in the field studies; better predictions were obtained for nonvegetated systems (relative errors between 0.4 and 9.7%) than for shaded-soil landscapes (relative errors between 2.3 and 27%). The model reflected field data showing that daily average emission rates of Hg-0, formed by the reduction of Hg(II), are primarily controlled by changes in solar radiation, soil moisture, temperature, and, to a lesser extent, wind conditions. The model may have potential use in several preliminary studies to characterize trends of airborne Hg emitted from terrestrial sources to the atmosphere. en
heal.publisher AIR & WASTE MANAGEMENT ASSOC en
heal.journalName JOURNAL OF THE AIR & WASTE MANAGEMENT ASSOCIATION en
dc.identifier.issue 3 en
dc.identifier.volume 52 en
dc.identifier.isi ISI:000174330000012 en
dc.identifier.spage 339 en
dc.identifier.epage 348 en


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